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I have not painted Icons yet, but I say a good airbrush with the right acrylic paints work best IMHO, see my thread should I should I not. I did a pair of Gas Can S in a matte finish. I scuffed (sanded) the frame and legs prior to applying my paint. Icons unless you have access or have paint adhesion promoter a light scuffing with sandpaper and followed by alcohol wash, should make for a good surface to start with. If you have not painted plastics or do not have your own airbrush and compressor, you may want to outsource the job. Because hobby paints and tactics can result in hobby looks and results.
I kind of want to do an "artist" series of icons for my new batwolfs coming in. But do you think sanding or stripping an icon would work best? Or maybe painting over a matte icon?
Sanding, no. Will introduce scratches that will need to be covered which means burying in more paint. I would suggest a light scuff with a scotch brite pad, then base them, mid coat if applicable, and clear. All depends on the end result you want.